Matches in SemOpenAlex for { <https://semopenalex.org/work/W4324367538> ?p ?o ?g. }
- W4324367538 endingPage "142413" @default.
- W4324367538 startingPage "142413" @default.
- W4324367538 abstract "Constructing the excellent rich-mesoporous carbon and exploring its electrosorption process are keys to promote the electrosorption industrialization of uranium. In this work, we develop a rich-mesoporous biocarbon by using alkali-thermal-pyrolysis and ammonia low-temperature plasma, and then systematically investigate its electrosorption kinetics and mechanism of U(VI) considering a series of Faradaic side reactions. After the above treatment, the electrosorption efficiency of U(VI) onto biocarbon improves from 49.75% to 94.45%, and the ultra-high U-selectivity coefficient (SU/M) is higher than 120 from the mixed solution. The kinetic diffusion process of U(VI) into the pores is crucial, even in different water systems. Importantly, Faradaic side reactions are proved to be non-negligible factors in the electrosorption of uranium. Especially, the oxygen reduction at the cathode can convert dissolved oxygen into H2O2, which oxides the amorphous electro-reduced U(V, IV) to U(VI), and finally forms crystalline uranium peroxide species. To sum up, this work not only offers an excellent uranium-selectivity electroadsorbent, but firstly confirms the influence of Faradaic side reactions that has been ignored in the current electrosorption of uranium." @default.
- W4324367538 created "2023-03-16" @default.
- W4324367538 creator A5004005455 @default.
- W4324367538 creator A5018228131 @default.
- W4324367538 creator A5035113720 @default.
- W4324367538 creator A5050493397 @default.
- W4324367538 creator A5059853801 @default.
- W4324367538 creator A5066258582 @default.
- W4324367538 creator A5079691564 @default.
- W4324367538 date "2023-05-01" @default.
- W4324367538 modified "2023-10-18" @default.
- W4324367538 title "The electrosorption of uranium (VI) onto the modified porous biocarbon with ammonia low-temperature plasma: Kinetics and mechanism" @default.
- W4324367538 cites W1906455749 @default.
- W4324367538 cites W1917802570 @default.
- W4324367538 cites W1966466023 @default.
- W4324367538 cites W1967676445 @default.
- W4324367538 cites W1996822951 @default.
- W4324367538 cites W2027917902 @default.
- W4324367538 cites W2030597363 @default.
- W4324367538 cites W2084826648 @default.
- W4324367538 cites W2088987441 @default.
- W4324367538 cites W2092766164 @default.
- W4324367538 cites W2127423008 @default.
- W4324367538 cites W2139002506 @default.
- W4324367538 cites W2162677524 @default.
- W4324367538 cites W2300733217 @default.
- W4324367538 cites W2343930434 @default.
- W4324367538 cites W2558302870 @default.
- W4324367538 cites W2559968893 @default.
- W4324367538 cites W2588853303 @default.
- W4324367538 cites W2600801254 @default.
- W4324367538 cites W2605020460 @default.
- W4324367538 cites W2610426651 @default.
- W4324367538 cites W2765431835 @default.
- W4324367538 cites W2770377455 @default.
- W4324367538 cites W2788422209 @default.
- W4324367538 cites W2810885672 @default.
- W4324367538 cites W2902214269 @default.
- W4324367538 cites W2903663661 @default.
- W4324367538 cites W2904807739 @default.
- W4324367538 cites W2905201690 @default.
- W4324367538 cites W2911620712 @default.
- W4324367538 cites W2915130917 @default.
- W4324367538 cites W2923123397 @default.
- W4324367538 cites W2936564142 @default.
- W4324367538 cites W2941671020 @default.
- W4324367538 cites W2945184931 @default.
- W4324367538 cites W2956656702 @default.
- W4324367538 cites W2982826361 @default.
- W4324367538 cites W2989820389 @default.
- W4324367538 cites W2994445201 @default.
- W4324367538 cites W3021834581 @default.
- W4324367538 cites W3022032034 @default.
- W4324367538 cites W3027251549 @default.
- W4324367538 cites W3035641541 @default.
- W4324367538 cites W3037401284 @default.
- W4324367538 cites W3087283490 @default.
- W4324367538 cites W3088588095 @default.
- W4324367538 cites W3109874456 @default.
- W4324367538 cites W3114694474 @default.
- W4324367538 cites W3118790623 @default.
- W4324367538 cites W3144369496 @default.
- W4324367538 cites W3164076544 @default.
- W4324367538 cites W3194190280 @default.
- W4324367538 cites W3196944409 @default.
- W4324367538 cites W3200213990 @default.
- W4324367538 cites W3207708614 @default.
- W4324367538 cites W3215136186 @default.
- W4324367538 cites W3216520151 @default.
- W4324367538 cites W4200036896 @default.
- W4324367538 cites W4200387764 @default.
- W4324367538 cites W4206516849 @default.
- W4324367538 cites W4214513644 @default.
- W4324367538 cites W4220941944 @default.
- W4324367538 cites W4221105503 @default.
- W4324367538 cites W4226180996 @default.
- W4324367538 cites W4281252502 @default.
- W4324367538 cites W4285227833 @default.
- W4324367538 cites W4291016496 @default.
- W4324367538 cites W4296890205 @default.
- W4324367538 cites W4310722123 @default.
- W4324367538 cites W4318617759 @default.
- W4324367538 doi "https://doi.org/10.1016/j.cej.2023.142413" @default.
- W4324367538 hasPublicationYear "2023" @default.
- W4324367538 type Work @default.
- W4324367538 citedByCount "6" @default.
- W4324367538 countsByYear W43243675382023 @default.
- W4324367538 crossrefType "journal-article" @default.
- W4324367538 hasAuthorship W4324367538A5004005455 @default.
- W4324367538 hasAuthorship W4324367538A5018228131 @default.
- W4324367538 hasAuthorship W4324367538A5035113720 @default.
- W4324367538 hasAuthorship W4324367538A5050493397 @default.
- W4324367538 hasAuthorship W4324367538A5059853801 @default.
- W4324367538 hasAuthorship W4324367538A5066258582 @default.
- W4324367538 hasAuthorship W4324367538A5079691564 @default.
- W4324367538 hasConcept C104779481 @default.
- W4324367538 hasConcept C118792377 @default.
- W4324367538 hasConcept C121332964 @default.