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- W43248846 abstract "A microbalance has been used to study the kinetics of the chemisorption of oxygen on cuprous oxide present as a layer on copper metal. The underlying copper enabled the surface to be regenerated reproducibly without excessive heat treatment, thereby minimizing sintering and changes in surface heterogeneity. Rates of chemisorption have been investigated on a single specimen between −70 and 60° and between 0.06 and 7.0 mm. The chemisorption can proceed to several monolayers and is largely irreversible. On the basis of the observed kinetics, it is concluded that the formation of the first monolayer proceeds with an activation energy of 7 kcal./mole, but thereafter the reaction enters a stage where the activation energy of the uptake steadily rises. The rate during this stage is considered to be controlled by a space charge produced in the surface layers as a result of the formation of cation vacancies. The suggested mechanism emphasizes the close relationship between this process and that of the oxidation of copper." @default.
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- W43248846 date "1957-01-01" @default.
- W43248846 modified "2023-10-18" @default.
- W43248846 title "47 Kinetics of the Chemisorption of Oxygen on Cuprous Oxide" @default.
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- W43248846 doi "https://doi.org/10.1016/s0360-0564(08)60196-0" @default.
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