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• W4327900623 abstract "Developing adsorptive separation processes based on C2 H6 -selective sorbents to replace energy-intensive cryogenic distillation is a promising alternative for C2 H4 purification from C2 H4 /C2 H6 mixtures, which however remains challenging. During our studies on two isostructural metal-organic frameworks (Ni-MOF 1 and Ni-MOF 2), we found that Ni-MOF 2 exhibited significantly higher performance for C2 H6 /C2 H4 separation than Ni-MOF-1, as clearly established by gas sorption isotherms and breakthrough experiments. Density-Functional Theory (DFT) studies showed that the unblocked unique aromatic pore surfaces within Ni-MOF 2 induce more and stronger C-H⋅⋅⋅π with C2 H6 over C2 H4 while the suitable pore spaces enforce its high C2 H6 uptake capacity, featuring Ni-MOF 2 as one of the best porous materials for this very important gas separation. It generates 12 L kg-1 of polymer-grade C2 H4 product from equimolar C2 H6 /C2 H4 mixtures at ambient conditions." @default.
• W4327900623 created "2023-03-21" @default.
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• W4327900623 date "2023-04-17" @default.
• W4327900623 modified "2023-10-17" @default.
• W4327900623 title "A Microporous Metal‐Organic Framework with Unique Aromatic Pore Surfaces for High Performance C₂H₆/C₂H₄ Separation" @default.
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• W4327900623 doi "https://doi.org/10.1002/anie.202302564" @default.
• W4327900623 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36940231" @default.
• W4327900623 hasPublicationYear "2023" @default.
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