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• W4327922441 endingPage "142505" @default.
• W4327922441 startingPage "142505" @default.
• W4327922441 abstract "A universal strategy to synthesize metal phosphides (MPs, M = Ni, Co, Cu, Fe, Pd, Pt, Ru) nanoparticles encapsulated in 2D defect-rich graphitic carbon shell (MPs@C-PPS) using P- and C-rich polymeric phosphide (PPS) as the precursor was brought out. Characterization results demonstrate that the thickness of the carbon shell on different MPs nanoparticles ranges from 1 to 7 nm, which can be adjusted by changing the Ni/P molar ratio. Some cracks and irregular defects are observed in carbon layers, which can selectively permeate small hydrogen molecules and block the passage of larger organic molecules. In catalytic performance test, the as-synthesized Ni2P@C-PPS exhibited excellent selectivity in alkynes semihydrogenation and high anti-sulfur poisoning and anti-acid corrosion capability in hydrogenation reactions. Mechanism exploration indicates that selective permeability of the carbon shell is the key to improving catalyst robustness." @default.
• W4327922441 created "2023-03-21" @default.
• W4327922441 creator A5039534717 @default.
• W4327922441 creator A5054358636 @default.
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• W4327922441 date "2023-05-01" @default.
• W4327922441 modified "2023-10-10" @default.
• W4327922441 title "Synthesis of metal phosphides encapsulated within defect carbon: A sulfur-tolerant and acid-resistant catalyst for selective hydrogenation" @default.
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• W4327922441 doi "https://doi.org/10.1016/j.cej.2023.142505" @default.
• W4327922441 hasPublicationYear "2023" @default.
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