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• W4327972783 endingPage "341091" @default.
• W4327972783 startingPage "341091" @default.
• W4327972783 abstract "Single-atom catalyst (SAC), one of the most attractive catalysts in the field of energy conversion and storage, was proven as efficient accelerator for luminol-dissolved oxygen electrochemiluminescence (ECL) via the catalysis of oxygen reduction reaction (ORR). In this work, we synthesized heteroatom doping SACs of Fe-N/P-C for the catalysis of cathodic luminol ECL. The doping of P could lower the reaction energy barrier of the OH* reduction, and promote catalytic efficiency toward ORR. The formation of reactive oxygen species (ROS) during ORR triggered cathodic luminol ECL. Greatly enhanced ECL emission catalyzed by SACs proved that Fe-N/P-C exhibited higher catalytic activity to ORR compared with Fe-N-C. Since the system was highly dependent on oxygen, an ultra-sensitive detection of a typical antioxidant, ascorbic acid, was achieved with detection limit of 0.03 nM. This study provides possibility to greatly enhance the performance of ECL platform through rational tailoring of SACs via heteroatom doping." @default.
• W4327972783 created "2023-03-21" @default.
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• W4327972783 date "2023-05-01" @default.
• W4327972783 modified "2023-10-14" @default.
• W4327972783 title "Single-atom boosted electrochemiluminescence via phosphorus doping of Fe–N/P–C catalysts" @default.
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• W4327972783 doi "https://doi.org/10.1016/j.aca.2023.341091" @default.
• W4327972783 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37005019" @default.
• W4327972783 hasPublicationYear "2023" @default.
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