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• W4328105035 abstract "Effective spatial separation and utilization of photogenerated charges are critical for photocatalysis process. Herein, novel Co3O4 @TiO2 @[email protected] double-shelled nanocage (CTCA) with spatially separated redox centers was synthesized by loading Co3O4 and Au NP cocatalysts on the inner and outer surfaces of Z-scheme heterojunction (TiO2 @CdS). The reduction rate constant of U(VI) by CTCA reached 0.218 min−1 under simulated sunlight irradiation, which was 6.6, 3.2 and 36.3 times than that of monolayer CTCA (0.033 min−1), CTC (0.068 min−1) and CT (0.006 min−1). The full-spectrum light-assisted photothermal catalytic performance can enable CTCA to remove 98.8% of U(VI) and degrade nearly 90% of five organic pollutants simultaneously. Detailed characterizations and theory calculations revealed that the photogenerated holes and electrons in CTCA flow inward and outward. More importantly, Co3O4 acts as a “nano heater” to generate the photothermal effect for further enhancing the charge transfer and accelerating the surface reaction kinetics. Meanwhile, the photogenerated electrons and superoxide radicals play a dominant role in reducing the adsorbed U(VI) to insoluble (UO2)O2·2H2O(s). This work provides valuable input toward a novel double-shelled hollow nanocage reactor with excellent photothermal catalysis ability for efficient recovery U(VI) from uranium mine wastewater to address environmental contamination issues." @default.
• W4328105035 created "2023-03-22" @default.
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• W4328105035 date "2023-06-01" @default.
• W4328105035 modified "2023-10-16" @default.
• W4328105035 title "Novel Co3O4@TiO2@CdS@Au double-shelled nanocage for high-efficient photocatalysis removal of U(VI): Roles of spatial charges separation and photothermal effect" @default.
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• W4328105035 doi "https://doi.org/10.1016/j.jhazmat.2023.131248" @default.
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