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- W4328114961 abstract "This work suggests an intriguing light-driven atomic assembly proposal to orderly configure the distribution of reactive sites to optimize the spin-entropy-related orbital interaction and charge transfer from electrocatalysts to intermediates. Herein, the introduced fluorine (F) atoms acting as photo-corrosion centres in MnO1.9F0.1 effectively soften the bonding interaction of Mn−O bonds in the IrCl3 solution. Therefore, partial Mn atoms can be successively replaced to form orderly atomic-hybridized catalysts with a spin-related low entropy due to the coexistence of Ir-atomic chains and clusters. The time-related elemental analysis demonstrates that the dynamic dissolution/redeposition of Ir clusters in acidic oxygen evolution leads to a reintegration of the reaction pathway to seek the switchable rate-limiting step with a lower activation energy." @default.
- W4328114961 created "2023-03-22" @default.
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- W4328114961 date "2023-04-14" @default.
- W4328114961 modified "2023-09-28" @default.
- W4328114961 title "Light‐driven Orderly Assembly of Ir‐atomic Chains to Integrate a Dynamic Reaction Pathway for Acidic Oxygen Evolution" @default.
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- W4328114961 doi "https://doi.org/10.1002/ange.202301128" @default.
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