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- W4328124161 abstract "Abstract The mechanisms involved in the oxidation of H 2 SO 4 to peroxydisulfuric acid (H 2 S 2 O 8 ) and H 2 O to O 2 on WO 3 , SnO 2 , and their interface models were investigated using density functional theory. Regardless of the metal oxide, the free energy changes for the two proton‐coupled electron transfer (PCET) steps of the H 2 SO 4 oxidation mechanism indicated that the first PCET is the rate‐limiting step that requires a greater energy input than the second one. Based on the free energy change in the rate‐limiting step, the WO 3 anode with SnO 2 was expected to produce electrochemically more H 2 S 2 O 8 in an aqueous H 2 SO 4 solution than SnO 2 only without O 2 evolution from H 2 O. We also experimentally confirmed that the Faraday efficiency of H 2 S 2 O 8 production using the WO 3 anode deposited on a F‐doped SnO 2 conductive glass (FTO) with lower applied potential is superior to FTO only." @default.
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- W4328124161 date "2023-03-21" @default.
- W4328124161 modified "2023-09-26" @default.
- W4328124161 title "Selective Oxidation of Sulfuric Acid to Peroxydisulfuric Acid on a Tungsten Trioxide Anode" @default.
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- W4328124161 doi "https://doi.org/10.1002/slct.202300114" @default.
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