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• W4328126046 abstract "Low safety, unstable interfaces, and high reactivity of liquid electrolytes greatly hinder the development of lithium metal batteries (LMBs). Quasi-solid-state electrolytes (QGPEs) with superior mechanical properties and high compatibility can meet the demands of LMBs. Herein, a biodegradable polyacrylonitrile/polylactic acid-block-ethylene glycol polymer (PALE) as membrane skeleton for GPEs is designed and systematically investigated by regulating the length and structure of the cross-linked chain. Benefiting from the enriched affinitive sites of polar functional groups (CO, COC, CN, and OH) in highly cross-linked polymer structure, the designed PALE membrane skeleton exhibits flame-retardant property and ultrahigh liquid electrolyte uptake property, and the derived quasi-solid-state PALE GPEs deliver enhanced stretchability and a higher electrochemical stable window of 5.11 V. Besides, the PALE GPEs effectively protect cathodes from corrosion while allowing uniform and fast transfer of Li+ ions. Therefore, the Li||Li symmetrical battery and LFP or NCM811||Li full-cell using PALE GPEs exhibit excellent cycling stability coupled with compact and flat inorganic/organic interface layers. And the excellent cycling stability of pouch cells under harsh operating conditions indicates the application possibilities of PALE GPEs in flexible devices with high-energy-density." @default.
• W4328126046 created "2023-03-22" @default.
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• W4328126046 date "2023-03-21" @default.
• W4328126046 modified "2023-10-15" @default.
• W4328126046 title "Regulation of Interphase Layer by Flexible Quasi‐Solid Block Polymer Electrolyte to Achieve Highly Stable Lithium Metal Batteries" @default.
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• W4328126046 doi "https://doi.org/10.1002/adfm.202300425" @default.
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