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• W4328130056 abstract "Transformation of CO2 into value-added chemicals remains a key challenge. Herein, nonthermal plasma (NTP)-activated CO2-H2O conversion over BaTiO3-mixed NiO/CeO2 (Ni/Ce+) and Co3O4/CeO2 (Co/Ce+) catalysts is demonstrated. In a continuous-flow dielectric barrier discharge reactor and under ambient conditions, optimum Co/Ce+ showed formation rates of CO and O2 of (43.6 ± 3.1) and (20.8 ± 0.7) μmol g−1h−1, respectively. CO2 conversion was found to be dependent on a combination of the basicity of the catalyst surface, CO2 flow rate, plasma input power, and relative humidity. Subsequently, kinetic analysis suggested that the activation energies over Ni/Ce+, Co/Ce+, and NiCo/Ce+ are 35.68, 15.61, and 25.88 kJ mol−1, respectively. By combining these findings, a plausible reaction mechanism that can facilitate understanding the trend of product formation is also provided." @default.
• W4328130056 created "2023-03-22" @default.
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• W4328130056 date "2023-04-19" @default.
• W4328130056 modified "2023-10-18" @default.
• W4328130056 title "Non‐thermal Plasma Assisted CO ₂ ‐H ₂ O Conversions over NiO and Co ₃ O ₄ supported on CeO ₂" @default.
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• W4328130056 doi "https://doi.org/10.1002/ceat.202200481" @default.
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