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- W4353092662 abstract "Abstract A direct and efficient carbon-sulfur bond formation method was developed. For the first time, cross-dehydrogenative-coupling (CDC) reaction of an especial type of benzyl ethers (isochroman) and a variety of thiols was investigated. 2,3-dichloro-5,6-dicyanobenzoquinone (DDQ) without using any metal catalyst provides a simple and efficient method to construct C-S bond leading to the library of sulfur-containing hetrocyclic compounds. Indeed, we can directly functionalize C sp3 -H bond by S-H bond without requiring pre-activation. As a result, this method will increase synthetic efficiency at the most fundamental level of organic synthesis." @default.
- W4353092662 created "2023-03-23" @default.
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- W4353092662 date "2023-03-22" @default.
- W4353092662 modified "2023-10-04" @default.
- W4353092662 title "DDQ-mediated direct cross-dehydrogenative-coupling (CDC) reaction of thiols with isochroman: A serendipitous metal-free route to C-S bond formation" @default.
- W4353092662 cites W2137590633 @default.
- W4353092662 doi "https://doi.org/10.21203/rs.3.rs-2609405/v1" @default.
- W4353092662 hasPublicationYear "2023" @default.
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