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- W4361014527 endingPage "4773" @default.
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- W4361014527 abstract "Prompted by the recent stepwise mechanistic proposal for the Huisgen [3+2] cycloaddition reaction between enamine and α-diazo ester, where the nucleophilic addition of the enamine carbon onto the terminal nitrogen of diazo ester is crucial, we examined the possible use of N-heterocyclic olefins (NHOs) as highly electron-rich dipolarophiles in these reactions. The mesoionic NHOs derived from 1,2,3-triazoles undergo fast [4+1] cycloaddition to give 3-(triazolium-4-yl)-(3H)-pyrazol-4-olates at room temperature. The reaction mechanism has been explored through experimental and DFT computational studies." @default.
- W4361014527 created "2023-03-30" @default.
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- W4361014527 date "2023-01-01" @default.
- W4361014527 modified "2023-10-18" @default.
- W4361014527 title "[4+1] cyclization of α-diazo esters and mesoionic N-heterocyclic olefins" @default.
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- W4361014527 doi "https://doi.org/10.1039/d3cc01139a" @default.
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