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• W4361018002 abstract "Utilizing advanced transmission electron microscopy (TEM), the structure at the (110)-type twin boundary (TB) of Ce-doped GdFeO3 (C-GFO) has been investigated with picometer precision. Such a TB is promising to generate local ferroelectricity within a paraelectric system, while precise knowledge about its structure is still largely missing. In this work, a direct measurement of the cation off-centering with respect to the neighboring oxygen is enabled by integrated differential phase contrast (iDPC) imaging, and up to 30 pm Gd off-centering is highly localized at the TB. Further electron energy loss spectroscopy (EELS) analysis demonstrates a slight accumulation of oxygen vacancies at the TB, a self-balanced behavior of Ce at the Gd sites, and a mixed occupation of Fe2+ and Fe3+ at the Fe sites. Our results provide an informative picture with atomic details at the TB of C-GFO, which is indispensable to further push the potential of grain boundary engineering." @default.
• W4361018002 created "2023-03-30" @default.
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• W4361018002 date "2023-03-27" @default.
• W4361018002 modified "2023-10-14" @default.
• W4361018002 title "Direct Visualization of Distorted Twin Boundaries in Ce-Doped GdFeO₃" @default.
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• W4361018002 doi "https://doi.org/10.1021/acs.nanolett.3c00318" @default.
• W4361018002 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36972518" @default.
• W4361018002 hasPublicationYear "2023" @default.
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