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• W4361228693 abstract "All-inorganic cesium lead triiodide (CsPbI3) perovskite has received increasing attention due to its intrinsic thermal stability and suitable band gap for photovoltaic applications. However, it is difficult to deposit high-quality pure-phase CsPbI3 films using CsI and PbI2 as precursors due to the rapid nucleation and crystal growth by the solution coating method. Here, a simple cation-exchange approach is employed to fabricate all-inorganic 3D CsPbI3 perovskite, where 1D ethylammonium lead (EAPbI3) perovskite is first solution-deposited and then transformed to 3D CsPbI3 via ion exchange between EA+ and Cs+ during thermal annealing. The large space between the PbI3– skeletons in 1D EAPbI3 favors the cation interdiffusion and exchange for the formation of pure-phase 3D CsPbI3 with full compactness and high crystallinity and orientation. The resulting CsPbI3 film exhibits a low trap density of state and high charge mobility, and the perovskite solar cell shows a power-conversion efficiency of 18.2% with enhanced stability. This strategy provides an alternative and promising fabrication route for the fabrication of high-quality all-inorganic perovskite devices." @default.
• W4361228693 created "2023-03-31" @default.
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• W4361228693 date "2023-03-29" @default.
• W4361228693 modified "2023-10-01" @default.
• W4361228693 title "Facile Dimension Transformation Strategy for Fabrication of Efficient and Stable CsPbI₃ Perovskite Solar Cells" @default.
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• W4361228693 doi "https://doi.org/10.1021/acsami.2c23289" @default.
• W4361228693 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36990658" @default.
• W4361228693 hasPublicationYear "2023" @default.
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