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• W4361285841 abstract "Dynamic materials undergoing adaptive solid-state transitions are attractive for soft mechanics and information technology. Here, we report a novel porous framework system based on macrocyclic trimers assembled from open-shell tetraarylethylene building blocks with aryldicyanomethyl radicals as coupling linkers. Under mechanical, thermal, or chemical stimuli, the framework showed adaptability by activating conformational dynamics and radical-based transformations, thus displaying macroscopic responsiveness in terms of light absorption, luminescence, and magnetism. We studied the dynamic processes by variable-temperature nuclear magnetic resonance (VT-NMR), variable-temperature electron spin resonance (VT-ESR), and superconducting quantum interference device (SQUID) measurement and further established a proof-of-concept application for multi-modal information encryption. The strategy may open avenues for rational design of solid-state photoelectromagnetic dynamic materials by merging dynamic covalent coupling chemistry and functional aggregation principles." @default.
• W4361285841 created "2023-03-31" @default.
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• W4361285841 date "2023-04-20" @default.
• W4361285841 modified "2023-10-17" @default.
• W4361285841 title "Photoelectromagnetic Responsive Adaptive Porous Frameworks through Dynamic Covalent Chemistry of Tetraarylethylene‐backboned Aryldicyanomethyl Radicals" @default.
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• W4361285841 doi "https://doi.org/10.1002/anie.202301719" @default.
• W4361285841 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36988141" @default.
• W4361285841 hasPublicationYear "2023" @default.
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