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• W4361286019 endingPage "131313" @default.
• W4361286019 startingPage "131313" @default.
• W4361286019 abstract "Nitrophenols (NPs) are highly toxic and easy to accumulate to high concentrations (> 500 mg/L) in real wastewater. The nitro group contained in NPs is an electron-absorbing group that is easy to reduce and difficult to oxidize, so there is an urgent need to develop reduction removal technology. Zero-valent aluminum (ZVAl) is an excellent electron donor that can reductively transform various refractory pollutants. However, ZVAl is prone to rapid deactivation due to non-selective reactions with water, ions, etc. To overcome this critical limitation, we prepared a new type of carbon nanotubes (CNTs) modified microscale ZVAl, [email protected], through a facile mechanochemical ball milling method. [email protected] had outstanding high reactivity in degrading p-nitrophenol even 1000 mg/L and showed up to 95.50% electron utilization efficiency. Moreover, [email protected] was highly resistant to the passivation by dissolved oxygen, ions and natural organic matters coexisting in water matrix, and remained highly reactive after aging in the air for 10 days. Furthermore, [email protected] could effectively remove dinitrodiazophenol from real explosive wastewater. The excellent performance of [email protected] is due to the combination of selective adsorption of NPs and CNTs-mediated e-transfer. [email protected] looks promising for the efficient and selective degradation of NPs, with broader prospects for real wastewater treatment." @default.
• W4361286019 created "2023-03-31" @default.
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• W4361286019 date "2023-06-01" @default.
• W4361286019 modified "2023-09-27" @default.
• W4361286019 title "Application potential of zero-valent aluminum in nitrophenols wastewater decontamination: Enhanced reactivity, electron selectivity and anti-passivation capability" @default.
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• W4361286019 doi "https://doi.org/10.1016/j.jhazmat.2023.131313" @default.
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