Matches in SemOpenAlex for { <https://semopenalex.org/work/W4361761774> ?p ?o ?g. }
- W4361761774 endingPage "7709" @default.
- W4361761774 startingPage "7703" @default.
- W4361761774 abstract "Understanding the growth and coarsening mechanisms of metal-organic framework (MOF) nanoparticles is crucially important for the design and fabrication of MOF materials with diverse functionalities and controllable stability. Oriented attachment (OA) growth is a common manner of MOF nanocrystal coarsening and agglomeration, but the underlying molecular mechanisms have not been well understood to date. Here we report the molecular-scale characterization of the OA interfaces of zeolitic imidazolate framework (ZIF) crystals by state-of-the-art low-dose aberration-corrected transmission electron microscopy. A series of OA interfaces with different molecular structures are captured, implying that multiple kinetic steps are involved in the OA growth of ZIF crystals from non-directional physical attractions between primary nanocrystals, lattice-aligned attachment of the ligand-capped nanocrystals, to coherent interfaces with perfect lattice alignment or stacking faults. It was found that the surface-capping organic ligands not only play an essential role in crystal lattice alignment by near-field directional interactions, but also dominate the interfacial reaction kinetics by interfacial diffusion-controlled elimination of excess surface-capping ligands. These observations provide molecular-scale insights into the OA growth mechanisms of ZIF crystals, which is important for engineering MOF crystal growth pathways by designing surface-capping ligands." @default.
- W4361761774 created "2023-04-04" @default.
- W4361761774 creator A5020565416 @default.
- W4361761774 creator A5025602649 @default.
- W4361761774 creator A5034264520 @default.
- W4361761774 creator A5040205022 @default.
- W4361761774 creator A5041129333 @default.
- W4361761774 creator A5055817822 @default.
- W4361761774 creator A5058283645 @default.
- W4361761774 creator A5059489499 @default.
- W4361761774 creator A5065014768 @default.
- W4361761774 creator A5067206054 @default.
- W4361761774 creator A5087266984 @default.
- W4361761774 creator A5087977210 @default.
- W4361761774 date "2023-01-01" @default.
- W4361761774 modified "2023-10-16" @default.
- W4361761774 title "Oriented attachment interfaces of zeolitic imidazolate framework nanocrystals" @default.
- W4361761774 cites W1677747913 @default.
- W4361761774 cites W1801166380 @default.
- W4361761774 cites W1971784141 @default.
- W4361761774 cites W1975501285 @default.
- W4361761774 cites W1980138378 @default.
- W4361761774 cites W1994460820 @default.
- W4361761774 cites W1999783956 @default.
- W4361761774 cites W1999908724 @default.
- W4361761774 cites W2001037711 @default.
- W4361761774 cites W2002799357 @default.
- W4361761774 cites W2004550299 @default.
- W4361761774 cites W2004692701 @default.
- W4361761774 cites W2010815579 @default.
- W4361761774 cites W2017582605 @default.
- W4361761774 cites W2021767761 @default.
- W4361761774 cites W2022167379 @default.
- W4361761774 cites W2027232636 @default.
- W4361761774 cites W2029050093 @default.
- W4361761774 cites W2048246447 @default.
- W4361761774 cites W2062773550 @default.
- W4361761774 cites W2068161718 @default.
- W4361761774 cites W2078115388 @default.
- W4361761774 cites W2082192143 @default.
- W4361761774 cites W2094145140 @default.
- W4361761774 cites W2113020843 @default.
- W4361761774 cites W2133562203 @default.
- W4361761774 cites W2133934213 @default.
- W4361761774 cites W2139482086 @default.
- W4361761774 cites W2141939342 @default.
- W4361761774 cites W2152495917 @default.
- W4361761774 cites W2163535530 @default.
- W4361761774 cites W2169899684 @default.
- W4361761774 cites W2221750675 @default.
- W4361761774 cites W2318363005 @default.
- W4361761774 cites W2321316383 @default.
- W4361761774 cites W2322392357 @default.
- W4361761774 cites W2329180172 @default.
- W4361761774 cites W2438516979 @default.
- W4361761774 cites W2511201702 @default.
- W4361761774 cites W2589811758 @default.
- W4361761774 cites W2609516724 @default.
- W4361761774 cites W2725088701 @default.
- W4361761774 cites W2752772741 @default.
- W4361761774 cites W2765767460 @default.
- W4361761774 cites W2769954071 @default.
- W4361761774 cites W2777639606 @default.
- W4361761774 cites W2783895701 @default.
- W4361761774 cites W2919258635 @default.
- W4361761774 cites W2945025851 @default.
- W4361761774 cites W2952828555 @default.
- W4361761774 cites W2963239459 @default.
- W4361761774 cites W3037481718 @default.
- W4361761774 cites W3111829433 @default.
- W4361761774 cites W3123022237 @default.
- W4361761774 cites W3127398570 @default.
- W4361761774 cites W3134114297 @default.
- W4361761774 cites W3149203567 @default.
- W4361761774 cites W3174701469 @default.
- W4361761774 cites W4293067736 @default.
- W4361761774 cites W582145995 @default.
- W4361761774 doi "https://doi.org/10.1039/d3nr00702b" @default.
- W4361761774 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37039237" @default.
- W4361761774 hasPublicationYear "2023" @default.
- W4361761774 type Work @default.
- W4361761774 citedByCount "2" @default.
- W4361761774 countsByYear W43617617742023 @default.
- W4361761774 crossrefType "journal-article" @default.
- W4361761774 hasAuthorship W4361761774A5020565416 @default.
- W4361761774 hasAuthorship W4361761774A5025602649 @default.
- W4361761774 hasAuthorship W4361761774A5034264520 @default.
- W4361761774 hasAuthorship W4361761774A5040205022 @default.
- W4361761774 hasAuthorship W4361761774A5041129333 @default.
- W4361761774 hasAuthorship W4361761774A5055817822 @default.
- W4361761774 hasAuthorship W4361761774A5058283645 @default.
- W4361761774 hasAuthorship W4361761774A5059489499 @default.
- W4361761774 hasAuthorship W4361761774A5065014768 @default.
- W4361761774 hasAuthorship W4361761774A5067206054 @default.
- W4361761774 hasAuthorship W4361761774A5087266984 @default.
- W4361761774 hasAuthorship W4361761774A5087977210 @default.
- W4361761774 hasConcept C146088050 @default.
- W4361761774 hasConcept C147789679 @default.