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- W4362466406 endingPage "109836" @default.
- W4362466406 startingPage "109836" @default.
- W4362466406 abstract "A series of metal oxide/ metal-organic frameworks (MOFs) composites ([email protected]/Ce-MOFs) were synthesized by partial thermal decomposition of Fe/Ce-MOFs which were synthesized with dielectric barrier discharge (DBD) plasma. The heterojunction interface between MOFs and metal oxides can effectively promote the electron interface transfer. When Fe was introduced, the energy band of the catalysts became narrower, and the increase of oxygen defects concentration slowed down the recombination rate of photogenerated electrons and holes, which greatly improved the photocatalytic performance. [email protected]/Ce-MOFs exhibited more efficient visible light photocatalytic performance than that of Fe/Ce-MOFs. [email protected]/Ce-MOFs-b (the molar ratio of Fe to Ce is 1:3) formed an abundant oxygen defect that facilitated the photocatalytic nitrogen fixation reaction. For [email protected]/Ce-MOFs-b, the NH4+ generation rate reached 299 μmol·L−1·h−1 after 2 h photoreaction under visible light with N2 and deionized water as solvent. Also, [email protected]/Ce-MOFs-b showed high cyclic stability. After three repeated cycles, the NH4+ generation rate maintained about 95%. This work provided a new method for the preparation of [email protected] and emphasized the importance of oxygen defects in nitrogen fixation." @default.
- W4362466406 created "2023-04-05" @default.
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- W4362466406 date "2023-06-01" @default.
- W4362466406 modified "2023-10-14" @default.
- W4362466406 title "DBD plasma assisted synthesis of MO@Fe/Ce-MOFs with rich oxygen defects as efficient photocatalysts for nitrogen fixation" @default.
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- W4362466406 doi "https://doi.org/10.1016/j.jece.2023.109836" @default.
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