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• W4362474911 abstract "Abstract To achieve environmentally benign energy conversion with the carbon neutrality target via electrochemical reactions, the innovation of electrocatalysts plays a vital role in the enablement of renewable resources. Nowadays, Pt-based nanocrystals (NCs) have been identified as one class of the most promising candidates to efficiently catalyze both the half-reactions in hydrogen- and hydrocarbon-based fuel cells. Here, we thoroughly discuss the key achievement in developing shape-controlled Pt and Pt-based NCs, and their electrochemical applications in fuel cells. We begin with a mechanistic discussion on how the morphology can be precisely controlled in a colloidal system, followed by highlighting the advanced development of shape-controlled Pt, Pt-alloy, Pt-based core@shell NCs, Pt-based nanocages, and Pt-based intermetallic compounds. We then select some case studies on models of typical reactions (oxygen reduction reaction at the cathode and small molecular oxidation reaction at the anode) that are enhanced by the shape-controlled Pt-based nanocatalysts. Finally, we provide an outlook on the potential challenges of shape-controlled nanocatalysts and envision their perspective with suggestions. Image missing<!-- image only, no MathML or LaTex -->" @default.
• W4362474911 created "2023-04-05" @default.
• W4362474911 creator A5011065863 @default.
• W4362474911 creator A5055440450 @default.
• W4362474911 creator A5076337939 @default.
• W4362474911 date "2023-03-31" @default.
• W4362474911 modified "2023-10-15" @default.
• W4362474911 title "Shape-Controlled Synthesis of Platinum-Based Nanocrystals and Their Electrocatalytic Applications in Fuel Cells" @default.
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