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- W4362502113 abstract "The ring-opening polymerization of β-lactones into polyhydroxyalkanoates (PHA), biodegradable polymers with high molecular weight and narrow polydispersity, is of significant interest. The mononuclear zirconium compound containing sterically hindered N,O-chelate and anionic dimethylamide ligands was used as an initiator for the polymerization of β-butyrolactone (BBL), resulting in polyhydroxylbutyrate (PHB) with a number-average molecular weight of 12 000 g mol-1. Kinetic studies demonstrate a first-order dependence on β-butyrolactone (BBL) concentration at room temperature, accompanied by narrow molecular weight distributions (ca. 1.03-1.07), indicating a well-controlled living polymerization." @default.
- W4362502113 created "2023-04-05" @default.
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- W4362502113 date "2023-01-01" @default.
- W4362502113 modified "2023-10-03" @default.
- W4362502113 title "Living ring-opening polymerization of β-butyrolactone initiated by mononuclear zirconium compounds containing sterically hindered <i>N</i>,<i>O</i>-chelate and anionic dimethylamide ligands" @default.
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- W4362502113 doi "https://doi.org/10.1039/d3ra00338h" @default.
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