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- W4362511538 abstract "Herein, we present our work on stepwise C—O/C—H activation with valence‐adjusted Ti‐complexes . The well‐designed [N 2 N] 2– ‐type ligands were able to support Ti‐center with different oxidation states, including +IV, +III, +II. Mechanistic studies revealed that the Ti II ‐species could activate THF by oxidative addition of C—O bond via a radical intermediate with the formation of a C sp 3 –Ti bond, while the corresponding Ti IV ‐alkyl species could activate C sp 2 –H bond via σ‐bond metathesis with a kitelike four‐centered Ti IV ‐transition state. This work may provide a unique strategy to generate the transition metal alkyl complex from the THF ring‐opening products. More details are discussed in the report by Shi et al . on page 1015—1022. image" @default.
- W4362511538 created "2023-04-06" @default.
- W4362511538 date "2023-04-01" @default.
- W4362511538 modified "2023-09-26" @default.
- W4362511538 title "Inside Cover Picture" @default.
- W4362511538 doi "https://doi.org/10.1002/cjoc.202390092" @default.
- W4362511538 hasPublicationYear "2023" @default.
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