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- W4362636745 abstract "All-organic aqueous batteries are deemed attractive energy storage systems for some application scenarios demanding recyclability or wearability. The efficient redox activity of quinone/hydroquinone-derived couples in biosystems inspires us to develop advanced batteries based on them. However, designing such an all-organic aqueous battery is challenging in selecting suitable electrolytes and active materials. A possible battery configuration consisting of the 9, 10-anthraquinone (AQ) anode, hydroquinone derivatives cathode, and weak acid metal-ion aqueous electrolyte is demonstrated herein. The molecular configuration of quinones and ionic type of electrolytes affect the redox behaviors of electrodes. Gratifyingly, a combination of AQ-tetrachlorohydroquinone-Al2(SO4)3 exhibits optimal performance. The underlying work mechanism of this full-battery configuration is disclosed by electrochemical and structural characterizations, finding that H+ and Al3+ are jointly involved in the redox reaction of quinone electrodes, and Al3+ plays a crucial role. This work inaugurates a new framework for designing an all-organic aqueous battery." @default.
- W4362636745 created "2023-04-07" @default.
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- W4362636745 date "2023-07-01" @default.
- W4362636745 modified "2023-10-15" @default.
- W4362636745 title "All-organic aqueous batteries consisting of quinone-hydroquinone derivatives with proton/aluminum-ion co-insertion mechanism" @default.
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- W4362636745 doi "https://doi.org/10.1016/j.apsusc.2023.157174" @default.
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