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• W4362693536 abstract "Iridium oxide is recognized as the best oxygen evolution anode material due to its excellent electrocatalytic activity and long-term stability in acidic environment. Electrodeposition, as a new method for preparing iridium oxide catalysts, has attracted extensive attention in recent years. We report a triangular-wave electrodeposition method for the preparation of iridium oxide electrodes and successfully synthesized highly active IrO x electrodes with ultralow iridium loading. The IrO x electrode prepared at 100 mV s −1 for 100 cycles exhibited a superior mass activity of 3.11 A mg Ir −1 , while the IrO x electrodeposited at 20 mV s −1 for 500 cycles has the best apparent electrocatalytic activity, Tafel slope as low as 54.75 mV dec −1 . Physical characterization and electrochemical experiments show that the calcination treatment plays an important role in enhancing the OER performance of the electrodes. Remarkably, the calcined IrO x -TWE/Ti can continuously catalyze OER in 0.5 M H 2 SO 4 at 50 mA cm −2 for 150 h with a slight performance decay, demonstrating a supper large stability number of <?CDATA $2.78times {10}^{5}.$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mn>2.78</mml:mn> <mml:mo>×</mml:mo> <mml:msup> <mml:mrow> <mml:mn>10</mml:mn> </mml:mrow> <mml:mn>5</mml:mn> </mml:msup> <mml:mo>.</mml:mo> </mml:math> This work provides some valuable insights into the application of electrodeposition-based iridium oxide to practical industrial systems." @default.
• W4362693536 created "2023-04-09" @default.
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• W4362693536 date "2023-04-01" @default.
• W4362693536 modified "2023-09-27" @default.
• W4362693536 title "A Study on the Triangular-Wave Electrodeposition of Iridium Oxide on Ti" @default.
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• W4362693536 doi "https://doi.org/10.1149/1945-7111/accb73" @default.
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