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- W4363650292 abstract "Comprehensive Summary Non‐halogenated polymers have great potential in the commercialization of organic solar cells (OSCs) due to their advantages in the manufacturing process. However, high‐performance donor polymers are limited to a small amount of building blocks. Herein, we utilize as building block 4 H ‐dithieno[3,2‐ e :2',3'‐ g ]isoindole‐4,6(5 H )‐dione (DTID) to design and synthesize a relevant non‐halogenated polymer PBTID for active layers in OSCs. PBTID exhibits a strong absorption in the wavelength range of 400—600 nm with a distinctly wide optical bandgap of 2.06 eV, a low‐lying highest occupied molecular orbital (HOMO) energy level of −5.53 eV. In addition, this polymer has a very strong aggregation effect in solution and could form nanoscale fibrils in the neat film. Consequently, when blended with the non‐fullerene acceptor Y6, the devices achieve a prominent PCE of 15.8% with a high V oc of 0.87 V. The V oc and PCE values are one of the highest values in the non‐halogenated polymer donor‐based OSCs reported to date." @default.
- W4363650292 created "2023-04-11" @default.
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- W4363650292 date "2023-05-17" @default.
- W4363650292 modified "2023-09-25" @default.
- W4363650292 title "A <scp>Non‐Halogenated</scp> Polymer Donor Based on Imide Unit for Organic Solar Cells with Efficiency Nearly 16%" @default.
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- W4363650292 doi "https://doi.org/10.1002/cjoc.202300007" @default.
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