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- W4365140220 abstract "Temporal delays extracted from photoionization phases are currently determined with attosecond resolution by using interferometric methods. Such methods require special care when photoionization occurs near Feshbach resonances due to the interference between direct ionization and autoionization. Although theory can accurately handle these interferences in atoms, in molecules, it has to face an additional, so far insurmountable problem: Autoionization is slow, and nuclei move substantially while it happens, i.e., electronic and nuclear motions are coupled. Here, we present a theoretical framework to account for this effect and apply it to evaluate time-resolved and vibrationally resolved photoelectron spectra and photoionization phases of N2 irradiated by a combination of an extreme ultraviolet (XUV) attosecond pulse train and an infrared pulse. We show that Feshbach resonances lead to unusual non-Franck-Condon vibrational progressions and to ionization phases that strongly vary with photoelectron energy irrespective of the vibrational state of the remaining molecular cation." @default.
- W4365140220 created "2023-04-13" @default.
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- W4365140220 date "2023-04-14" @default.
- W4365140220 modified "2023-10-18" @default.
- W4365140220 title "Attosecond photoionization delays in the vicinity of molecular Feshbach resonances" @default.
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- W4365140220 doi "https://doi.org/10.1126/sciadv.ade3855" @default.
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