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- W4365509566 abstract "Multivalent ions in solutions with polyelectrolytes (PE) induce electrostatic correlations that can drastically change ion distributions around the PEs and their mutual interactions. Using coarse-grained molecular dynamics simulations, we show how in addition to valency, ion shape and concentration can be harnessed as tools to control like-charged PE-PE interactions. We demonstrate a correlation between the orientational ordering of aspherical ions and how they mediate the effective PE-PE attraction induced by multivalency. The interaction type, strength, and range can thus be externally controlled in ionic solutions. Our results can be used as generic guidelines to tune the self-assembly of like-charged polyelectrolytes by variation of the characteristics of the ions." @default.
- W4365509566 created "2023-04-15" @default.
- W4365509566 creator A5047081153 @default.
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- W4365509566 date "2023-04-14" @default.
- W4365509566 modified "2023-10-16" @default.
- W4365509566 title "Interactions between Rigid Polyelectrolytes Mediated by Ordering and Orientation of Multivalent Nonspherical Ions in Salt Solutions" @default.
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- W4365509566 doi "https://doi.org/10.1103/physrevlett.130.158202" @default.
- W4365509566 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37115871" @default.
- W4365509566 hasPublicationYear "2023" @default.
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