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- W4366122005 abstract "In the current article, the effect of Si/Al ratio on the NOx adsorption and storage capacity over Pd/Beta with 1 wt% Pd loading was investigated. The XRD, 27Al NMR and 29Si NMR measurements were used to determine the structure of Pd/Beta zeolites. XAFS, XPS, CO-DRIFT, TEM and H2-TPR were used to identify the Pd species. The results showed that the NOx adsorption and storage capacity on Pd/Beta zeolites gradually decreased with the increase of Si/Al ratio. Pd/Beta-Si (Si-rich, Si/Al~260) rarely has NOx adsorption and storage capacity, while Pd/Beta-Al (Al-rich, Si/Al~6) and Pd/Beta-C (Common, Si/Al~25) exhibit excellent NOx adsorption and storage capacity and suitable desorption temperature. Pd/Beta-C has slightly lower desorption temperature compared to Pd/Beta-Al. The NOx adsorption and storage capacity increased for Pd/Beta-Al and Pd/Beta-C by hydrothermal aging treatment, while the NOx adsorption and storage capacity on Pd/Beta-Si had no change." @default.
- W4366122005 created "2023-04-19" @default.
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- W4366122005 date "2023-04-16" @default.
- W4366122005 modified "2023-09-30" @default.
- W4366122005 title "Effects of Si/Al Ratio on Passive NOx Adsorption Performance over Pd/Beta Zeolites" @default.
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- W4366122005 doi "https://doi.org/10.3390/molecules28083501" @default.
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