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• W4366132017 abstract "Abstract Faradaic reactions including charge transfer are often accompanied with diffusion limitation inside the bulk. Conductive two‐dimensional frameworks (2D MOFs) with a fast ion transport can combine both—charge transfer and fast diffusion inside their porous structure. To study remaining diffusion limitations caused by particle morphology, different synthesis routes of Cu‐2,3,6,7,10,11‐hexahydroxytriphenylene (Cu 3 (HHTP) 2 ), a copper‐based 2D MOF, are used to obtain flake‐ and rod‐like MOF particles. Both morphologies are systematically characterized and evaluated for redox‐active Li + ion storage. The redox mechanism is investigated by means of X‐ray absorption spectroscopy, FTIR spectroscopy and in situ XRD. Both types are compared regarding kinetic properties for Li + ion storage via cyclic voltammetry and impedance spectroscopy. A significant influence of particle morphology for 2D MOFs on kinetic aspects of electrochemical Li + ion storage can be observed. This study opens the path for optimization of redox active porous structures to overcome diffusion limitations of Faradaic processes." @default.
• W4366132017 created "2023-04-19" @default.
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• W4366132017 date "2023-05-17" @default.
• W4366132017 modified "2023-10-14" @default.
• W4366132017 title "Overcoming Diffusion Limitation of Faradaic Processes: Property‐Performance Relationships of 2D Conductive Metal‐Organic Framework Cu₃(HHTP)₂ for Reversible Lithium‐Ion Storage" @default.
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• W4366132017 doi "https://doi.org/10.1002/anie.202303111" @default.
• W4366132017 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37069123" @default.
• W4366132017 hasPublicationYear "2023" @default.
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