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- W4366163676 abstract "Although mixed-matrix membranes (MMMs) have been extensively studied, their commercial applications have been hampered by scientific and engineering challenges. Herein, we report an innovative one-step MMM fabrication method that can put the commercialization of MMMs forward by overcoming most of the current challenges because it enables the rapid formation of high-performance asymmetric MMMs in a scalable manner. The method termed phase-inversion in sync with metal–organic framework (MOF) formation (PIMOF) involves a polymer film undergoing phase inversion and simultaneously ZIF-8 nanoparticles forming in-situ inside the polymer. The resulting MMMs show unexpectedly high C3H6/C3H8 separation performances (C3H6 permeance of ca. 7.5 GPU and C3H6/C3H8 separation factor of ca. 107), which is attributed mostly to the high effective ZIF-8 loading (>50 wt%) and the enhanced molecular sieving effect of the unusually small sub-5 nm ZIF-8 filler nanoparticles by restricted linker motion." @default.
- W4366163676 created "2023-04-19" @default.
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- W4366163676 date "2023-06-01" @default.
- W4366163676 modified "2023-10-13" @default.
- W4366163676 title "Highly propylene-selective asymmetric mixed-matrix membranes by polymer phase-inversion in sync with in-situ ZIF-8 formation" @default.
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- W4366163676 doi "https://doi.org/10.1016/j.cej.2023.143048" @default.
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