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- W4366238172 abstract "Quantum interference (QI) dominates the electronic properties of single molecules even at room temperature and can lead to a large change in their electrical conductance. To take advantage of this for nanoelectronic applications, a mechanism to electronically control QI in single molecules needs to be developed. In this paper, we demonstrate that controlling the quantum interference of each spin in a stable open-shell organic radical with a large π-system is possible by changing the spin state of the radical. We show that the counterintuitive constructive spin interference in a meta-connected radical changes to destructive interference by changing the spin state of the radical from a doublet to a singlet. This results in a significant change in the room temperature electrical conductance by several orders of magnitude, opening up new possibilities for spin interference based molecular switches for energy storage and conversion applications." @default.
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- W4366238172 date "2023-04-18" @default.
- W4366238172 modified "2023-10-09" @default.
- W4366238172 title "Controlling Spin Interference in Single Radical Molecules" @default.
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- W4366238172 doi "https://doi.org/10.1021/acs.nanolett.2c05068" @default.
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