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• W4366251512 abstract "A series of X%Cu/SAPO-34 (X = 1.0, 2.0, 4.0 and 6.0) catalysts were prepared by ultrasonic impregnation method for selective catalytic reduction (SCR) of NOx with ammonia. The effect of different Cu loadings on the selective catalytic reduction of NO by molecular sieve catalysts was examined on a fixed-bed reactor. Catalyst physicochemical properties were characterized and analyzed using XRD, TEM, NH3-TPD, H2-TPR, and in situ DRIFTS. Catalysts were used in reaction kinetics studies from the perspective of transient and steady-state kinetics. Cu/SAPO-34 catalyst with 4% Cu loading had the best denitrification efficiency and wide activity window. Copper species were highly dispersed on the catalyst surface. Cu/SAPO-34 catalyst with 4% Cu loading had rich acidic sites and excellent redox performance. Cu/SAPO-34 catalysts with 4% Cu loading possess minimal activation energy and were lower than commercial catalysts. According to the results of in situ IR, transient and steady-state analysis, the Cu/SAPO-34 catalyst with 4% Cu loading in the NH3-SCR reaction process was mainly E-R mechanism, and there was L-H mechanism." @default.
• W4366251512 created "2023-04-20" @default.
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• W4366251512 date "2023-04-18" @default.
• W4366251512 modified "2023-09-25" @default.
• W4366251512 title "Effect of Cu loading on the performance and kinetics of Cu/SAPO-34 catalysts for selective catalytic reduction with NH3" @default.
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• W4366251512 doi "https://doi.org/10.1007/s11356-023-26957-8" @default.
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