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- W4366352146 abstract "Peroxide dianion (O22-) has strong oxidizing activity and ease of proton abstraction and is extremely unstable. Direct and controllable adsorption and release of O22- has large application implication and is a large challenge so far. Here, we use a unique metal (Ni)-organic (diphenylalanine, DPA) framework (MOF), Ni(DPA)2, as adsorbents for absorption and release of O22-. This MOF structure has room-temperature magnetoelectricity via distortion of the Ni-centered octahedron {NiN2O4} and thus possesses a tunable ferroelectric polarization under applied electric/magnetic fields. Controllable adsorption and release of O22- are realized in such a MOF system via electrochemical redox measurements. Structural/spectroscopic characterization and calculations reveal that a number of NH active sites in the nanopores of MOF can effectively adsorb O22- by hydrogen bonds and then tunable ferroelectric polarization induces controllable release of O22- under applied magnetic fields. This work presents a constructive way for controllable adsorption and release of reactive oxygen species." @default.
- W4366352146 created "2023-04-21" @default.
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- W4366352146 date "2023-04-19" @default.
- W4366352146 modified "2023-10-16" @default.
- W4366352146 title "Magnetoelectricity-Mediated Tunable Absorption and Release of Peroxide Dianions" @default.
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- W4366352146 doi "https://doi.org/10.1021/acs.nanolett.2c04803" @default.
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