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- W4366371911 abstract "The intimate host-anion interactions will regulate thermodynamics and kinetics in the self-assembly of cationic cages mimicking biological counterparts. Herein, we report construction and transformation of three Pd(II)-based metal-organic cages (MOCs) depending on different anions. Stoichiometric conversions of the lantern-shaped MOC-34 into either octahedral MOC-35 or tricapped trigonal prism MOC-36 are induced by BF4‒ or NO3‒, respectively. MOC-36 is kinetically favored and can undergo quantitative conversion to the thermodynamically preferred MOC-35 upon heating, accelerated by excess BF4‒ to motivate dissociative dynamics of Pd-vertices and lower activation barrier of cage transformation. The guest encapsulation behaviors of MOC-35 and MOC-36 have also been tested. These results manifest a significance of host-anion dynamics beyond complementary anion template, shedding light on the understanding of intricate anion recognition in nature." @default.
- W4366371911 created "2023-04-21" @default.
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- W4366371911 date "2023-04-01" @default.
- W4366371911 modified "2023-09-27" @default.
- W4366371911 title "Anion-induced differential assembly and structural transformation of supramolecular coordination cages" @default.
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- W4366371911 doi "https://doi.org/10.1016/j.cclet.2023.108477" @default.
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