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- W4366442067 endingPage "100608" @default.
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- W4366442067 abstract "The replacement of traditional functional groups with polycyclic scaffolds has been increasingly rewarding in medicinal chemistry programs. Over the decades, 1,3-disubstituted bicyclo[1.1.1]pentanes (BCPs) have demonstrated the potential for being competent bioisosteres for aryl-, alkyl- and alkynyl substructures. Although highly desired, mild and versatile synthetic methods to access synthetically valuable BCP-containing building blocks remain limited. Herein, a versatile way to access bridgehead substituted BCP nitriles, a useful BCP building block, is described, enabled by the unexpected selectivity of nickel in the multi-component radical cyanation. Commodity materials including carboxylic acids, amines, sulfonyl chlorides, and alkyl chlorides are engaged to provide a broad spectrum of substituted BCP nitriles in a single-step, multi-component fashion." @default.
- W4366442067 created "2023-04-21" @default.
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- W4366442067 date "2023-05-01" @default.
- W4366442067 modified "2023-10-18" @default.
- W4366442067 title "Nickel-mediated alkyl-, acyl-, and sulfonylcyanation of [1.1.1]propellane" @default.
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- W4366442067 doi "https://doi.org/10.1016/j.checat.2023.100608" @default.
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