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• W4366446732 abstract "Abstract Herein we report the thermodynamic and transport properties of a polymer-DES solution. The density, apparent viscosity, electrical conductivity, and interfacial tension for the mixtures of poly (ethylene glycol) (PEG)/zinc chloride (ZnCl 2 )/ethylene glycol (EG) with various compositions were determined experimentally in the temperature range of 303.15 to 343.15 K. The variations of density, apparent viscosity, electrical conductivity, and interfacial tension with the temperature, PEG concentration, molar ratio of ZnCl 2 to EG, and PEG molecular weight were analyzed and interpreted with the variations of H-bond, molecular thermal motion, polymer chain “end” effect, and polymer chain entanglement. The results showed that the hydrogen bond effect displayed enhancement with molar ratio of ZnCl 2 /EG and weakening with temperature, PEG concentration and molecular weight. The polymer chain “end” effect was enhanced with PEG concentration and weakened with PEG molecular weight. The effect of polymer chain entanglement was enhanced with PEG concentration and molecular weight. At low temperatures the Zn 2+ -EG H-bond was stronger than Zn 2+ -PEG while the situation became opposite at high temperatures. The correlations of density, apparent viscosity, and electrical conductivity with temperature and correlation of viscosity with density were conducted and the results showed that the activation energy of viscosity E η showed increase while the activation energy of conductivity E κ displayed decrease with the molar ratio of ZnCl 2 /EG and the closed-packed volumes of the PEG/ZnCl 2 /EG mixtures displayed increases with PEG concentration." @default.
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• W4366446732 date "2023-04-19" @default.
• W4366446732 modified "2023-10-16" @default.
• W4366446732 title "Density, apparent viscosity, electrical conductivity, interfacial tension, and intermolecular interactions of PEG-ZnCl2-EG solution" @default.
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• W4366446732 doi "https://doi.org/10.21203/rs.3.rs-2822566/v1" @default.
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