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• W4366464238 abstract "Abstract The electrolysis of dilute CO 2 streams suffers from low concentrations of dissolved substrate and its rapid depletion at the electrolyte‐electrocatalyst interface. These limitations require first energy‐intensive CO 2 capture and concentration, before electrolyzers can achieve acceptable performances. For direct electrocatalytic CO 2 reduction from low‐concentration sources, we introduce a strategy that mimics the carboxysome in cyanobacteria by utilizing microcompartments with nanoconfined enzymes in a porous electrode. A carbonic anhydrase accelerates CO 2 hydration kinetics and minimizes substrate depletion by making all dissolved carbon available for utilization, while a highly efficient formate dehydrogenase reduces CO 2 cleanly to formate; down to even atmospheric concentrations of CO 2 . This bio‐inspired concept demonstrates that the carboxysome provides a viable blueprint for the reduction of low‐concentration CO 2 streams to chemicals by using all forms of dissolved carbon." @default.
• W4366464238 created "2023-04-22" @default.
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• W4366464238 date "2023-05-12" @default.
• W4366464238 modified "2023-10-17" @default.
• W4366464238 title "Carboxysome‐Inspired Electrocatalysis using Enzymes for the Reduction of CO₂ at Low Concentrations**" @default.
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• W4366464238 doi "https://doi.org/10.1002/anie.202218782" @default.
• W4366464238 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37078435" @default.
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