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- W4366495148 abstract "The semiconductor phase molybdenum disulfide (2H-MoS2) with poor hydrogen evolution reaction (HER) performance restricts the further improvement of hydrogen production. Herein, an acetic acid coupled structure phase engineering (SPE) strategy is developed to synthesize a homogeneous and orderly cobalt molybdenum composite structure. The resulting CoS2/MoS2 complexes reveal excellent HER activity with a low overpotential of 80, 95, and 135 mV at 10 mA cm−2 in 0.5 M H2SO4, 1 M KOH, and 1 M PBS. Fourier transform infrared spectroscopy (FT-IR) and thermogravimetry mass spectrometry (TGA-MS) results illustrate that acetic acid is successfully coupled at the interface between CoS2 and MoS2. Results from density functional theory demonstrate that the π-π conjunction formed by acetic acid coupling can work as a bridge to help electrons transfer from cobalt to molybdenum. More importantly, the method can be extended to the synthesis of other composite materials with the similar structure." @default.
- W4366495148 created "2023-04-22" @default.
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- W4366495148 date "2023-09-01" @default.
- W4366495148 modified "2023-10-09" @default.
- W4366495148 title "Structure phase engineering strategy through acetic acid coupling to boost hydrogen evolution reaction performance of 2H phase MoS2 at wide pH range" @default.
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- W4366495148 doi "https://doi.org/10.1016/j.fuel.2023.128428" @default.
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