FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4366496088> ?p ?o ?g. }

• W4366496088 endingPage "3463" @default.
• W4366496088 startingPage "3454" @default.
• W4366496088 abstract "Conventional thermal annealing, known as the entropy-mediated strategy, is commonly used in directing the self-assembly of DNA-functionalized gold nanoparticles (DNA–AuNPs). The enthalpy-mediated strategy is another tractable approach, which can circumvent metastability by controlling the dynamic pathways at a condition with temperature remaining constant. However, the lack of direct measurements and observations of the assembly processes limits our understanding of the mechanism of how the systems avoid kinetic trapping and realize the phase transition successfully. In this work, we introduce a toy model for the self-assembly of DNA–AuNPs, which suggests that using the enthalpy-mediated strategy can effectively avoid undesired defects during the self-assembly. The effectiveness of this strategy in directing the self-assembly is proved through coarse-grained molecular dynamics simulations of DNA–AuNPs, which achieve the crystallization through orderly structural transformations. On the basis of that, we study the assembly processes which are controlled by enthalpy-mediated and entropy-mediated strategies. The DNA–AuNPs in the self-assembly controlled by the entropy-mediated strategy organize themselves during the thermal annealing process and are slowly frozen to achieve the crystallization. In contrast, we find that DNA–AuNPs in the primary stage of self-assembly which is controlled by the enthalpy-mediated strategy experience an organization–breakdown–reorganization process before forming stable crystallites, highlighting the importance of bond reversibility in the structural transitions and in avoiding the kinetic traps." @default.
• W4366496088 created "2023-04-22" @default.
• W4366496088 creator A5019658342 @default.
• W4366496088 creator A5033284358 @default.
• W4366496088 creator A5072777093 @default.
• W4366496088 date "2023-04-20" @default.
• W4366496088 modified "2023-10-15" @default.
• W4366496088 title "Avoiding Kinetic Trapping in the Self-Assembly of DNA-Functionalized Gold Nanoparticles by Using an Enthalpy-Mediated Strategy" @default.
• W4366496088 cites W1588463119 @default.
• W4366496088 cites W1617520624 @default.
• W4366496088 cites W1974083574 @default.
• W4366496088 cites W1978375794 @default.
• W4366496088 cites W1980301976 @default.
• W4366496088 cites W1986325765 @default.
• W4366496088 cites W1986677755 @default.
• W4366496088 cites W2009963235 @default.
• W4366496088 cites W2010590839 @default.
• W4366496088 cites W2015131862 @default.
• W4366496088 cites W2032434705 @default.
• W4366496088 cites W2041658612 @default.
• W4366496088 cites W2042024815 @default.
• W4366496088 cites W2053784498 @default.
• W4366496088 cites W2064294810 @default.
• W4366496088 cites W2065537227 @default.
• W4366496088 cites W2068350472 @default.
• W4366496088 cites W2069507241 @default.
• W4366496088 cites W2077139454 @default.
• W4366496088 cites W2083571075 @default.
• W4366496088 cites W2083579241 @default.
• W4366496088 cites W2092204065 @default.
• W4366496088 cites W2097041808 @default.
• W4366496088 cites W2108149882 @default.
• W4366496088 cites W2121563903 @default.
• W4366496088 cites W2125371586 @default.
• W4366496088 cites W2128899338 @default.
• W4366496088 cites W2130138775 @default.
• W4366496088 cites W2132706746 @default.
• W4366496088 cites W2136166668 @default.
• W4366496088 cites W2144835432 @default.
• W4366496088 cites W2154459955 @default.
• W4366496088 cites W2155727418 @default.
• W4366496088 cites W2172114355 @default.
• W4366496088 cites W2253375036 @default.
• W4366496088 cites W2256021634 @default.
• W4366496088 cites W2268896324 @default.
• W4366496088 cites W2310933479 @default.
• W4366496088 cites W2321813557 @default.
• W4366496088 cites W2461107267 @default.
• W4366496088 cites W2464689993 @default.
• W4366496088 cites W2519723230 @default.
• W4366496088 cites W2520643498 @default.
• W4366496088 cites W2606380959 @default.
• W4366496088 cites W2610856665 @default.
• W4366496088 cites W2756453057 @default.
• W4366496088 cites W2773368957 @default.
• W4366496088 cites W2810268565 @default.
• W4366496088 cites W2888066961 @default.
• W4366496088 cites W2892062634 @default.
• W4366496088 cites W2897347098 @default.
• W4366496088 cites W2902888941 @default.
• W4366496088 cites W2949451139 @default.
• W4366496088 cites W3010223142 @default.
• W4366496088 cites W3016189615 @default.
• W4366496088 cites W3027419250 @default.
• W4366496088 cites W3031479504 @default.
• W4366496088 cites W3087399847 @default.
• W4366496088 cites W3098739554 @default.
• W4366496088 cites W3101081102 @default.
• W4366496088 cites W3101861338 @default.
• W4366496088 cites W3104941576 @default.
• W4366496088 cites W3105840559 @default.
• W4366496088 cites W3135918615 @default.
• W4366496088 cites W4238327249 @default.
• W4366496088 cites W4362127574 @default.
• W4366496088 cites W4362235795 @default.
• W4366496088 cites W2186876778 @default.
• W4366496088 doi "https://doi.org/10.1021/acs.macromol.2c02204" @default.
• W4366496088 hasPublicationYear "2023" @default.
• W4366496088 type Work @default.
• W4366496088 citedByCount "0" @default.
• W4366496088 crossrefType "journal-article" @default.
• W4366496088 hasAuthorship W4366496088A5019658342 @default.
• W4366496088 hasAuthorship W4366496088A5033284358 @default.
• W4366496088 hasAuthorship W4366496088A5072777093 @default.
• W4366496088 hasConcept C104819515 @default.
• W4366496088 hasConcept C106301342 @default.
• W4366496088 hasConcept C121332964 @default.
• W4366496088 hasConcept C155672457 @default.
• W4366496088 hasConcept C159467904 @default.
• W4366496088 hasConcept C159985019 @default.
• W4366496088 hasConcept C171250308 @default.
• W4366496088 hasConcept C178790620 @default.
• W4366496088 hasConcept C185592680 @default.
• W4366496088 hasConcept C192562407 @default.
• W4366496088 hasConcept C203036418 @default.
• W4366496088 hasConcept C26856880 @default.
• W4366496088 hasConcept C2777855556 @default.
• W4366496088 hasConcept C3288061 @default.

• next