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- W4366807482 abstract "Abstract A highly enantioselective tandem Michael addition of tryptamine‐derived oxindoles to alkynones was developed by taking advantage of a chiral N , N′ ‐dioxide Sc(OTf) 3 catalyst. The reaction enables the facile preparation of enantioenriched spiro[pyrrolidine‐3,3′‐oxindole] compounds, which provides a novel strategy for the synthesis of monoterpenoid indole alkaloids. As a demonstration, the asymmetric synthesis of strychnos alkaloids [(−)‐tubifoline, (−)‐tubifolidine, (−)‐dehydrotubifoline] was achieved in 10–11 steps." @default.
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- W4366807482 date "2018-02-28" @default.
- W4366807482 modified "2023-10-15" @default.
- W4366807482 title "Highly Enantioselective Tandem Michael Addition of Tryptamine-Derived Oxindoles to Alkynones: Concise Synthesis of Strychnos Alkaloids" @default.
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- W4366807482 doi "https://doi.org/10.1002/anie.201800567" @default.
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