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• W4366824905 startingPage "143174" @default.
• W4366824905 abstract "The rational deposition of active atomic cocatalysts onto the exposing facets of photocatalysts is challenging. Herein, following the theoretical guidance, Pt single atoms (SAs) and Ni nanoclusters (NCs) have been introduced onto the (0 0 1) facet and a small amount of Ni clusters have been introduced are deposited on (1 0 1) facet of hydrogenated TiO2 nanosheets by a room temperature H2/Ar plasma method. The resulted H-TiO2@Pt SAs-Ni NCs exhibits high-performance solar hydrogen evolution with a rate of 71 mmol/g/h. Photoelectrochemical tests and theoretical simulation show that the introducing Ni-Pt brings about new external energy levels, elevates the valence band and suppresses the recombination of photo-generated electrons and holes. The computational results confirm that the H-O bond of the adsorbed H2O molecule was significantly activated on the Pt SAs-TiO2, and Ni NCs-TiO2. The co-promotion effect of Pt SAs and Ni NCs facilitates the enhanced performance. This work provides new opportunity for the design of advanced crystal facet-induced engineering nano-catalysts." @default.
• W4366824905 created "2023-04-25" @default.
• W4366824905 creator A5000653140 @default.
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• W4366824905 date "2023-06-01" @default.
• W4366824905 modified "2023-10-10" @default.
• W4366824905 title "Engineering hydrogenated TiO2 nanosheets by rational deposition of Ni clusters and Pt single atoms onto exposing facets for high-performance solar fuel production" @default.
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• W4366824905 doi "https://doi.org/10.1016/j.cej.2023.143174" @default.
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