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- W4366977404 startingPage "143139" @default.
- W4366977404 abstract "ReO4−, as a typical anion, its capture is now receiving increasing attentions. However, there still lacks effective method to boost the uptake performance of materials, except for designing new materials. In this work, we found that the structural flexibility could be a good candidate to boost ReO4− uptake. The used flexible cationic MOF, [Co(H2O)2(TIB)][NO3]2 (named as Co-TIB-NO3, TIB = 3,3′,5,5′-tetra(1H-imidazol-1-yl)-1,1′-biphenyl), showed a multiple response towards temperature, counterion, and solvents with the observation of three different structures, including crystalline OP (open pore) phase, crystalline CP (closed pore) phase, and amorphous CP phase. The origin of the structural flexibility is quite complicated, involving a cage-to-channel migration for counterion, interlayer compression, and deformation of organic ligands. The developed material, Co-TIB-NO3-313, showing the amorphous CP phase, was found to perform outstanding ReO4− capture with a high uptake capacity, rapid adsorption rate, large distribution coefficient, excellent selectivity, and recyclability, suggesting its superior application in ReO4− capture." @default.
- W4366977404 created "2023-04-27" @default.
- W4366977404 creator A5001469778 @default.
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- W4366977404 date "2023-06-01" @default.
- W4366977404 modified "2023-10-17" @default.
- W4366977404 title "Structural flexibility in cationic metal–organic framework for boosting ReO4− capture" @default.
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- W4366977404 doi "https://doi.org/10.1016/j.cej.2023.143139" @default.
- W4366977404 hasPublicationYear "2023" @default.
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