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- W4366992200 abstract "A new approach is presented here for constructing higher-performance anion exchange membranes (AEMs) by combining block-type and comb-shaped architectures. A series of quaternization fluorene-containing block poly (arylene ether nitrile ketone)s (QFPENK-m-n) were synthesized by varying the length of hydrophobic segment as AEMs. The well-designed architecture, which involved grafting comb-shaped C10 long alkyl side chains onto the block-type main chains, formed efficient ion-transport channels, as confirmed by atomic force microscopy. As a result, the AEMs showed high hydroxide conductivities in the range of 34.3–102.1 mS⋅cm−1 from 30 to 80 °C at moderate ion exchange capacities (IECs). Moreover, the hydrophobic segment with nitrile groups also exhibited a profound anti-swelling property for the AEMs, resulting in ultralow swelling ratios ranging from 4.7% to 7.1% at 30 °C and 7.5%–9.8% at 80 °C, as well as superb conductivity-to-swelling ratios at 80 °C. In addition, the AEMs displayed good mechanical properties, thermal and oxidative stability, and optimizable alkaline stability." @default.
- W4366992200 created "2023-04-27" @default.
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- W4366992200 date "2023-08-01" @default.
- W4366992200 modified "2023-09-25" @default.
- W4366992200 title "Block poly(arylene ether nitrile ketone)s with comb-shaped alkyl chains as anion exchange membranes" @default.
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- W4366992200 doi "https://doi.org/10.1016/j.ijhydene.2023.03.472" @default.
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