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• W4366993092 abstract "To explore novel two-dimensional superconductors, the recently prepared biphenylene network (BPN) monolayer with alkaline metal adatoms was investigated theoretically. Our study suggests that the superconducting critical temperature (Tc) of BPN monolayer could be increased from 0.03 to 11.22 K by adsorption of Li atoms, which induces increased density of states at the Fermi Level, softened vibrations and electron pockets at the Fermi surface. The diffusion barrier of Li/Na adatoms is very low (<0.25 eV), and it tends to decrease for high coverage. Average conductance was proposed to quantitatively evaluate the intrinsic conductivity and electronic transport anisotropy of two-dimensional materials. The adsorption of alkaline metal atoms enhances the transport anisotropy more than twice, and the direction with better conductance derives from the connected delocalized multi-center π bonds. Our study suggests that adsorption of metal atoms is an effective way to functionalize BPN monolayers, which endows them potential applications in future superconducting and electronic devices. It also implies that carbon monolayer allotropes like BPN monolayer may provide good platforms for both fundamental research and device applications, which stimulates more explorations in various fields." @default.
• W4366993092 created "2023-04-27" @default.
• W4366993092 creator A5007661109 @default.
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• W4366993092 date "2023-08-01" @default.
• W4366993092 modified "2023-09-25" @default.
• W4366993092 title "Superconducting and transport properties of biphenylene network monolayer with alkaline metal adatoms" @default.
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• W4366993092 doi "https://doi.org/10.1016/j.apsusc.2023.157255" @default.
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