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• W4367153003 abstract "The template-based design of the crystal structure is a direct and highly efficient method to achieve optimal nonlinear optical (NLO, meaning second-order NLO) performances. The structural flexibility of porous salt-inclusion chalcogenides (SICs) provides an alternative platform for modulating the enlargement of the band gap (that is generally positive with laser-induced damage threshold) and second harmonic generation (SHG) response simultaneously. By applying the pore reconstruction strategy to SIC [K3Cl][Mn2Ga6S12] (1), a new derivative K3Rb3[K3Cl][Li2Mn4Ga12S27] (2) is successfully isolated, which unusually features a heterologous nanopore framework with inner diameters of 8.90 and 9.16 Å. Guided by such a strategy, compound 2 possesses the widest band gap (3.31 eV) among the magnetic NLO chalcogenides; this finding is dominantly attributed to the porous structure and the dimensional deduction effect. Moreover, phase 2 displays a remarkable phase-matchable SHG intensity (1.1 × AgGaS2 at the incident laser of 1910 nm) that originated from the oriented alignment of NLO-functional motifs, as well as the rich terminal S atoms in the nanopore structure. Furthermore, the pore reconstruction strategy offers an efficient pathway to explore potential NLO candidates with excellent comprehensive performances; in particular, it settles the conflicting issue of enhancing the band gap (>3.0 eV) and SHG intensity (>1.0 × AgGaS2) concurrently." @default.
• W4367153003 created "2023-04-28" @default.
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• W4367153003 date "2023-01-01" @default.
• W4367153003 modified "2023-10-18" @default.
• W4367153003 title "Breaking the bottleneck of simultaneously wide band gap and large nonlinear optical coefficient by a “pore reconstruction” strategy in a salt-inclusion chalcogenide" @default.
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• W4367153003 doi "https://doi.org/10.1039/d3mh00389b" @default.
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