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• W4367307574 abstract "Abstract Three linear isoelectronic conjugated polymers PCC , PBC , and PBN are synthesized by Suzuki‐Miyaura polycondensation for photocatalytic hydrogen (H 2 ) production from water. PBN presented an excellent photocatalytic hydrogen evolution rate (HER) of 223.5 µmol h −1 (AQY 420 = 23.3%) under visible light irradiation, which is 7 times that of PBC and 31 times that of PCC . The enhanced photocatalytic activity of PBN is due to the improved charge separation and transport of photo‐induced electrons/holes originating from the lower exciton binding energy ( E b ), longer fluorescence lifetime, and stronger built‐in electric field, caused by the introduction of the polar B←N unit into the polymer backbone. Moreover, the extension of the visible light absorption region and the enhancement of surface catalytic ability further increase the activity of PBN . This work reveals the potential of B←N fused structures as building blocks as well as proposes a rational design strategy for achieving high photocatalytic performance." @default.
• W4367307574 created "2023-04-29" @default.
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• W4367307574 date "2023-04-28" @default.
• W4367307574 modified "2023-10-17" @default.
• W4367307574 title "Replacing CC Unit with B←N Unit in Isoelectronic Conjugated Polymers for Enhanced Photocatalytic Hydrogen Evolution" @default.
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• W4367307574 doi "https://doi.org/10.1002/smll.202302384" @default.
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