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• W4367309504 abstract "In contrast to ensemble-averaged measurements, single-molecule experiments directly display the heterogeneity of molecular properties in space and time. In many complex systems, spatial heterogeneity is regularly accompanied by temporal or dynamic heterogeneity; if a property differs from molecule to molecule, it will often vary in time for one and the same molecule. In this short paper, we discuss a few examples of complex systems where dynamical heterogeneity was observed in single-molecule or single-particle optical signals. For single biomolecules, the first demonstration of dynamic heterogeneity in a single enzyme was provided by Xie and colleagues. Other examples are found in glassy systems, and very recently in the magnetic relaxation of single superparamagnetic nanoparticles. The ubiquity of this phenomenon suggests that, rather than an exception, dynamic heterogeneity is the rule in complex systems with multiple degrees of freedom." @default.
• W4367309504 created "2023-04-29" @default.
• W4367309504 creator A5065097100 @default.
• W4367309504 date "2023-04-28" @default.
• W4367309504 modified "2023-09-30" @default.
• W4367309504 title "Dynamic Heterogeneity in the Optical Signals from Single Nano-Objects" @default.
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• W4367309504 doi "https://doi.org/10.1021/acs.jpcb.2c09055" @default.
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• W4367309504 hasPublicationYear "2023" @default.
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