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• W4367395617 abstract "Although it is generally accepted by the perovskite solar cells community that their interface behaviors have a profound impact on their power conversion efficiency (PCE) and stability, such interfacial engineering on the bottom interface between electron transport layer (ETL) and perovskite film is still lagging. Herein, a 3D graphene (G)–CuInS 2 composite is designed as an efficient ETL to improve both the interfacial contact and passivate defects at the G–CuInS 2 /perovskite interface. The lattice matching of graphene and methylammonium lead iodide CH 3 NH 3 PbI 3 inhibits the concentrated stress generated during the growth of perovskite, resulting in crystal films with large grain boundaries. The low‐electron defect density in 3D G–CuInS 2 composite facilitates the electron transport from perovskite film to CuInS 2 quantum dots. In addition, 3D G–CuInS 2 shows excellent carrier extraction capability of reducing carrier extraction time by 1.47 times than that of the counterpart. Correspondingly, a highly improved PCE of 22.4% is obtained, which increases by 15% of the counterpart. Furthermore, the unencapsulated device based on 3D G–CuInS 2 shows long‐term stability, maintaining 85% of its original efficiency in air for 30 days. This strategy provides a new route to interfacial passivation engineering for preparation of high‐performance perovskite solar cells." @default.
• W4367395617 created "2023-04-30" @default.
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• W4367395617 date "2023-05-10" @default.
• W4367395617 modified "2023-10-01" @default.
• W4367395617 title "New Insights into Interfacial Passivation on 3D Graphene–CuInS₂ Composites‐Based Perovskite Solar Cells" @default.
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• W4367395617 doi "https://doi.org/10.1002/solr.202300166" @default.
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