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• W4367669540 abstract "sp2 carbon-conjugated covalent organic framework (sp2 c-COF) featured with high π-conjugation, high chemical stabilities, and designable chemical structures, are thus promising for applications including adsorption and separation, optoelectronic devices, and catalysis. For the most of these applications, large-area and continuous films are required. However, due to the needs of harsh conditions in the formation of CC bonds, classical interfacial methodologies are challenged in the synthesis of sp2 c-COFs films. Herein, a novel and robust interfacial method namely copper-surface-mediated Knoevenagel polycondensation (Cu-SMKP), is shown for scalable synthesis of sp2 c-COF films on various Cu substrates. Using this approach, large-area and continuous sp2 c-COF films could be prepared on various complicated Cu surfaces with thickness from tens to hundreds of nanometers. The resultant sp2 c-COF films on Cu substrate could be used directly as functional electrode for extraction of uranium from spiked seawater, which gives an exceptionally uptake capacity of 2475 mg g-1 . These results delineate significant synthetic advances in sp2 c-COF films and implemented them as functional electrodes for uranyl capture." @default.
• W4367669540 created "2023-05-03" @default.
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• W4367669540 date "2023-05-02" @default.
• W4367669540 modified "2023-10-17" @default.
• W4367669540 title "Synthesis of sp² Carbon‐Conjugated Covalent Organic Framework Thin‐Films via Copper‐Surface‐Mediated Knoevenagel Polycondensation" @default.
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• W4367669540 doi "https://doi.org/10.1002/smll.202207972" @default.
• W4367669540 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37129557" @default.
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