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- W4367670587 abstract "In this work, we report a series of single-component molecules crystals named dialkyl 4,4′-oxalyldibenzoate (n-BZ) with both efficient room temperature phosphorescence (RTP) emission, multilevel stimuli responsiveness, and elasticity or flexibility. The crystalline n-BZ will change from original RTP single emission to RTP dual emission after grinding or thermal annealing (TA). Interestingly, the emission wavelength difference between the RTP dual-emission peaks after grinding or TA reaches 82 nm with emission color changes from cyan blue to orange. In addition, to our knowledge, the largest RTP quantum yield of 25.1% (6-BZ) has been achieved as the highest recorded for organic RTP elastic crystals. Through a series of experiments and theoretical calculations, we demonstrate that the multilevel stimuli responsiveness of n-BZ originates from the transition of excited state conformation and its elasticity from many weak intermolecular interactions, which will provide a molecular design and construction strategy for organic stimuli-responsive RTP materials." @default.
- W4367670587 created "2023-05-03" @default.
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- W4367670587 date "2023-06-01" @default.
- W4367670587 modified "2023-10-13" @default.
- W4367670587 title "An elastic organic crystal with multilevel stimuli-responsive room temperature phosphorescence" @default.
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- W4367670587 doi "https://doi.org/10.1016/j.matt.2023.04.006" @default.
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