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- W4368347761 abstract "Electrochemical carbon dioxide reduction reaction (CO2RR) is an effective approach to capture CO2 and convert it into value-added chemicals and fuels, thereby reducing excess CO2 emissions. Recent reports have shown that copper-based catalysts exhibit excellent performance in converting CO2 into multi-carbon compounds and hydrocarbons. However, the selectivity to the coupling products is poor. Therefore, tuning CO2-reduction selectivity toward C2+ products over Cu-based catalyst is one of the most important issues in CO2RR. Herein, we prepare a nanosheet catalyst with interfaces of Cu0/Cu+. The catalyst achieves Faraday efficiency (FE) of C2+ over 50% in a wide potential window between − 1.2 V to − 1.5 V versus reversible hydrogen electrode (vs. RHE). Moreover, the catalyst exhibits maximum FE of 44.5% and 58.9% towards C2H4 and C2+, with a partial current density of 10.5 mA cm−2 at − 1.4 V. Density functional theory (DFT) calculations show that the interface of Cu0/Cu+ facilitates CC coupling to form C2+ products, while inhibits CO2 conversion to C1 products." @default.
- W4368347761 created "2023-05-05" @default.
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- W4368347761 date "2023-09-01" @default.
- W4368347761 modified "2023-09-28" @default.
- W4368347761 title "Creating interfaces of Cu0/Cu+ in oxide-derived copper catalysts for electrochemical CO2 reduction to multi-carbon products" @default.
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- W4368347761 doi "https://doi.org/10.1016/j.jcis.2023.04.133" @default.
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